If you don't feel like climbing the actual volcano you can leave for a small hike uphill (not to bad) before sunrise, you will leave by car which will take you to the beginning of the trail. You get to the top for sunrise and see a spectacular view of lake atitlan as well as the smoking San Pedro Volcano. We booked this through our hostel - Casa Blanca GH at the end of the main lower road.
I'm sure you can book it elsewhere.
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