We used the Bondi and Sydney explorer buses which I would highly recommend but found the blue mountains version nowhere near as informative or good value. You really only need about 5 stops of the 25 and stops 1-9 are just one high street. Once you get into the mountains it was more useful and the book provided had good suggestions for walks and things to look at and the driver had some good information and ideas. The mountains and scenery are truly spectacular and well worth a day trip from Sydney. Again the last 8-10 stops didn't have much more than the high street of the next town. My issue was the price of 38 dollars each which really only involved 3 bus journeys of about 5km. Seeing as the return train to the blue mountains costs 11 dollars I felt this was a real rip off. If there is a group of you look into renting a car it will probably be cheaper
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