I definitely recommend taking the ring tram around this area first. Take a good look of the area, the buildings, the streets, and make a list of which ones you like the most. Then definitely take a tour on foot around this area, taking into account what you've listed, spend more time in those places. It is a very lovely area to walk, especially in good weather, the streets are almost empty in some regions and if you want to walk peacefully without being interrupted by hordes of tourists. The architecture is lovely and it lifts your heart up just to look around, enjoy the tall trees and the streets. Definitely the best feature of Vienna.
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