Brooklyn is a borough (New York City is made up of 5 boroughs) that contains many neighborhoods; Greenwich Village is a neighborhood in the borough of Manhattan. So what you want is a tour that covers both some Brooklyn neighborhoods and Greenwich Village. One that I know of that does that is the "All Loops" tour on the Gray Line bus. Here's a link to the page on their site that describes the tour, costs, etc.:
Thanks Crans that's just what we are looking for, perfect.
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