Ancient Thira is set high on top of a peninsula between the towns Kamari and Perissa. It has stunning panoramic views as you walk through the ancient town. The ruins are very interesting and have a number of information boards throughout - although not enough in my opinion if attending without a tour guide. Be aware, there are no toilets or cafes up top (not on the day I went anyway). If you're keen for a good hike, walking up the winding road from Kamari is a great exercise with lovely views the whole way!
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